Hank Azaria character Gargamel
Neil Patrick Harris character Patrick Winslow
Jayma Mays character Grace Winslow
Sofía Vergara character Odile Anjelou
Katy Perry character Smurfette (voice)
Madison McKinley character Model
Meg Phillips character Model
Mahadeo Shivraj character Cabbie
Frank Welker character Azrael (voice)
Tim Gunn character Henri
Julie Chang character Newscaster
Roger Clark character Newscaster
Mark Doherty character Bluetooth Businessman
Minglie Chen character Young Woman
Sean Kenin character Guy in Plaid Shirt
Victor Pagan character Bum
Adria Baratta character Anjelou Employee
Paula Pizzi character Odile's Mother
Andrew Sellon character Waiter
Julianna Rigoglioso character Little Sister
Daria Rae Figlo character Blonde Sister
Bradley Gosnell character Toy Salesperson
Heidi Armbruster character Toy Store Parent
Finnerty Steeves character Toy Store Parent
John Speredakos character Parent with Girls
Skai Jackson character Kicking Girl
Alex Hall character Skateboard Kid
Eric Redgate character Skateboard Kid
Jojo Gonzalez character FAO Custodian
Scott Dillin character Cop
Tyree Michael Simpson character Cop
Sean Ringgold character Inmate Bubba
Mario D'Leon character Bubba's Inmate Friend
Liz Smith character Party Guest
Tom Colicchio character Party Guest
Michael Musto character Party Guest
Joan Rivers character Party Guest
Olivia Palermo character Party Guest
Julia Enescu character Party Guest
Lauren Waggoner character Party Guest
Mr. Krinkle character Azrael
Hank character Elway
Jonathan Winters character Papa Smurf (voice)
Alan Cumming character Gutsy Smurf (voice)
Fred Armisen character Brainy Smurf (voice)
George Lopez character Grouchy Smurf (voice)
Anton Yelchin character Clumsy Smurf (voice)
Kenan Thompson character Greedy Smurf (voice)
Jeff Foxworthy character Handy Smurf (voice)
John Oliver character Vanity Smurf (voice)
Wolfgang Puck character Chef Smurf (voice)
Gary Basaraba character Hefty Smurf (voice)
Paul Reubens character Jokey Smurf (voice)
B.J. Novak character Baker Smurf (voice)
Tom Kane character Narrator Smurf (voice)
John Kassir character Crazy Smurf (Voice)
Joel McCrary character Farmer Smurf (voice)
Mary McGloin character Mother of Girl in Store (uncredited)
