Sean Connery character James Bond
Daniela Bianchi character Tatiana "Tanja" Romanova
Lotte Lenya character Rosa Klebb
Bernard Lee character M
Desmond Llewelyn character Q
Lois Maxwell character Miss Moneypenny
Pedro Armendáriz character Ali Kerim Bey
Robert Shaw character Donovan 'Red' Grant
Vladek Sheybal character Kronsteen
Eunice Gayson character Sylvia Trench
Walter Gotell character Morzeny
Francis de Wolff character Vavra
Nadja Regin character Kerim's Girl
Aliza Gur character Vida
George Pastell character Train Conductor (uncredited)
Martine Beswick character Zora
Jan Williams character Masseuse
Peter Madden character McAdams
Anthony Dawson character Ernst Blofeld
Hasan Ceylan character Foreign Agent (uncredited)
Neville Jason character Kerim's Chauffeur (uncredited)
Peter Bayliss character Benz (uncredited)
Nusret Ataer character Mehmet (uncredited)
Peter Brayham character Rhoda (uncredited)
Julie Mendez character Girl Dancing During Opening Titles (uncredited)
Bill Brandon character Gypsy (uncredited)
Moris Farhi character Gypsy (uncredited)
Alf Mangan character Gypsy (uncredited)
Dido Plumb character Gypsy (uncredited)
Ernie Rice character Gypsy (uncredited)
Fred Wood character Gypsy (uncredited)
Andre Charisse character Hotel Concierge (uncredited)
Hugo de Vernier character Hotel Porter (uncredited)
Victor Harrington character Chess Tournament Spectator (uncredited)
Barbara Jefford character Tatiana Romanova (voice) (uncredited)
Jim O'Brady character Krilencu's Henchman (uncredited)
Eric Pohlmann character Ernst Stavro Blofeld (voice) (uncredited)
Bob Simmons character James Bond in Gunbarrel Sequence (uncredited)
Gordon Sterne character SPECTRE Helicopter Pilot (uncredited)
Nikki Van der Zyl character Sylvia Trench / Receptionist (voice) (uncredited)
Pat Ryan character Naval Officer Listening to Bond's Tape (uncredited)
Michael Culver character Man in a Punt (uncredited)
Elizabeth Counsell character Woman in a Punt (uncredited)
Bedri Çavusoglu character Police (uncredited)